Spin Resolution and Evidence for Superexchange on NiO(001) Observed by Force Microscopy

Pielmeier, Florian and Giessibl, Franz J. (2013) Spin Resolution and Evidence for Superexchange on NiO(001) Observed by Force Microscopy. PHYSICAL REVIEW LETTERS, 110 (26): UNSP 26610. ISSN 0031-9007,

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Abstract

The spin order of the nickel oxide (001) surface is resolved, employing noncontact atomic force microscopy at 4.4 K using bulk Fe and SmCo tips mounted on a qPlus sensor that oscillates at sub-50 pm amplitudes. The spin-dependent signal is hardly detectable with Fe tips. In contrast, SmCo tips yield a height contrast of 1.35 pm for Ni ions with opposite spins. SmCo tips even show a small height contrast on the O atoms of 0.5 pm within the 2 x 1 spin unit cell, pointing to the observation of superexchange. We attribute the increased signal-to-noise ratio to the increased magnetocrystalline anisotropy energy of SmCo, which stabilizes the magnetic moment at the apex. Atomic force spectroscopy on the Ni up arrow, Ni down arrow, and O lattice site reveals a magnitude of the exchange energy of merely 1 meV at the closest accessible distance with an exponential decay length of lambda(exe) = 18 pm.

Item Type: Article
Uncontrolled Keywords: ATOMIC-RESOLUTION; MAGNETIC-MOMENTS; SURFACE; NIO(100); IMAGES; TIP;
Subjects: 500 Science > 530 Physics
Divisions: Physics > Institute of Experimental and Applied Physics > Chair Professor Giessibl > Group Franz J. Giessibl
Depositing User: Dr. Gernot Deinzer
Date Deposited: 07 Apr 2020 11:44
Last Modified: 07 Apr 2020 11:44
URI: https://pred.uni-regensburg.de/id/eprint/16493

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