Exciton broadening in WS2/graphene heterostructures

Hill, Heather M. and Rigosi, Albert F. and Raja, Archana and Chernikov, Alexey and Roquelet, Cyrielle and Heinz, Tony F. (2017) Exciton broadening in WS2/graphene heterostructures. PHYSICAL REVIEW B, 96 (20): 205401. ISSN 2469-9950, 2469-9969

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Abstract

We have used optical spectroscopy to observe spectral broadening of WS2 exciton reflectance peaks in heterostructures of monolayer WS2 capped with mono- to few-layer graphene. The broadening is found to be similar for the A and B excitons and on the order of 5-10 meV. No strong dependence on the number of graphene layers was observed within experimental uncertainty. The broadening can be attributed to charge- and energy-transfer processes between the two materials, providing an observed lower bound for the corresponding time scales of 65 fs.

Item Type: Article
Uncontrolled Keywords: DER-WAALS HETEROSTRUCTURES; TRANSITION-METAL DICHALCOGENIDES; MONOLAYER MOS2; ENERGY-TRANSFER; 2-DIMENSIONAL MATERIALS; CHARGE-TRANSFER; VALLEY POLARIZATION; TUNGSTEN DISULFIDE; ELECTRIC-FIELD; LAYER MOS2;
Subjects: 500 Science > 530 Physics
Divisions: Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Depositing User: Dr. Gernot Deinzer
Date Deposited: 14 Dec 2018 13:19
Last Modified: 28 Feb 2019 10:05
URI: https://pred.uni-regensburg.de/id/eprint/1971

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