Ultrafast electron diffraction from nanophotonic waveforms via dynamical Aharonov-Bohm phases

Mohler, K. J. and Ehberger, D. and Gronwald, I and Lange, C. and Huber, R. and Baum, P. (2020) Ultrafast electron diffraction from nanophotonic waveforms via dynamical Aharonov-Bohm phases. SCIENCE ADVANCES, 6 (47): eabc8804. ISSN 2375-2548,

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Abstract

Electron interferometry via phase-contrast microscopy, holography, or picodiffraction can provide a direct visualization of the static electric and magnetic fields inside or around a material at subatomic precision, but understanding the electromagnetic origin of light-matter interaction requires time resolution as well. Here, we demonstrate that pump-probe electron diffraction with all-optically compressed electron pulses can capture dynamic electromagnetic potentials in a nanophotonic material with sub-light-cycle time resolution via centrosymmetry-violating Bragg spot dynamics. The origin of this effect is a sizable quantum mechanical phase shift that the electron de Broglie wave obtains from the oscillating electromagnetic potentials within less than 1 fs. Coherent electron imaging and scattering can therefore reveal the electromagnetic foundations of light-matter interaction on the level of the cycles of light.

Item Type: Article
Uncontrolled Keywords: ELECTROMAGNETIC POTENTIALS; MICROSCOPY; HOLOGRAPHY;
Subjects: 500 Science > 530 Physics
Divisions: Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Depositing User: Dr. Gernot Deinzer
Date Deposited: 08 Mar 2021 09:53
Last Modified: 08 Mar 2021 09:53
URI: https://pred.uni-regensburg.de/id/eprint/43461

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