Phonon-Dominated Energy Transport in Purely Metallic Heterostructures

Herzog, Marc and von Reppert, Alexander and Pudell, Jan-Etienne and Henkel, Carsten and Kronseder, Matthias and Back, Christian H. and Maznev, Alexei A. and Bargheer, Matias (2022) Phonon-Dominated Energy Transport in Purely Metallic Heterostructures. ADVANCED FUNCTIONAL MATERIALS, 32 (41): 2206179. ISSN 1616-301X, 1616-3028

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Abstract

Ultrafast X-ray diffraction is used to quantify the transport of energy in laser-excited nanoscale gold-nickel (Au-Ni) bilayers. Electron transport and efficient electron-phonon coupling in Ni convert the laser-deposited energy in the conduction electrons within a few picoseconds into a strong non-equilibrium between hot Ni and cold Au phonons at the bilayer interface. Modeling of the subsequent equilibration dynamics within various two-temperature models confirms that for ultrathin Au films, the thermal transport is dominated by phonons instead of conduction electrons because of the weak electron-phonon coupling in Au.

Item Type: Article
Uncontrolled Keywords: LATTICE-DYNAMICS; ELECTRON; SOLIDS; heterostructures; nanoscale energy transports; non-equilibrium; thermal transports; ultrafast phenomena
Subjects: 500 Science > 530 Physics
Divisions: Physics > Institute of Experimental and Applied Physics
Depositing User: Dr. Gernot Deinzer
Date Deposited: 02 Feb 2024 07:05
Last Modified: 02 Feb 2024 07:05
URI: https://pred.uni-regensburg.de/id/eprint/58272

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