Coherent acoustic phonons in a coupled hexagonal boron nitride-graphite heterostructure

Ungeheuer, Arne and Bach, Nora and Mir, Mashood T. and Hassanien, Ahmed S. and Noeding, Lukas and Baumert, Thomas and Schaefer, Sascha and Senftleben, Arne (2024) Coherent acoustic phonons in a coupled hexagonal boron nitride-graphite heterostructure. STRUCTURAL DYNAMICS-US, 11 (1): 014501. ISSN 2329-7778

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Abstract

Femtosecond optically excited coherent acoustic phonon modes (CAPs) are investigated in a free-standing van der Waals heterostructure composed of a 20-nm transparent hexagonal boron nitride (hBN) and a 42-nm opaque graphite layer. Employing ultrafast electron diffraction, which allows for the independent evaluation of strain dynamics in the constituent material layers, three different CAP modes are identified within the bilayer stack after the optical excitation of the graphite layer. An analytical model is used to discuss the creation of individual CAP modes. Furthermore, their excitation mechanisms in the heterostructure are inferred from the relative phases of these modes by comparison with a numerical linear-chain model. The results support an ultrafast heat transfer mechanism from graphite to the hBN lattice system, which is important to consider when using this material combination in devices.

Item Type: Article
Uncontrolled Keywords: ULTRAFAST ELECTRON CRYSTALLOGRAPHY; STRUCTURAL DYNAMICS; GENERATION; DIFFRACTION; GRAPHENE
Subjects: 500 Science > 530 Physics
Divisions: Physics > Institute of Experimental and Applied Physics
Depositing User: Dr. Gernot Deinzer
Date Deposited: 30 Oct 2025 05:58
Last Modified: 30 Oct 2025 05:58
URI: https://pred.uni-regensburg.de/id/eprint/64729

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